Well if you have a Classic Controller or Gamecube controller, I STRONGLY suggest getting Super Mario 64 (N64) or Super Mario World (SNES), if you don't own them. Mario 64 is in my top 5 favourite games of all time.
If you don't have those controllers, try Super Mario Bros (NES) or Super Mario Bros 3 (NES), those are my 2 favourite games of all time.
It may seem weird just suggesting Mario, but his platformers are hands down the best on the VC, IMO.
Zelda Ocarina of Time (N64) and Kirby's Adventure (NES) are also great.

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